One Chemical Revolution or Three?

Rethinking Chemistry's History Through Multiple Transformations

Exploring the three fundamental transformations that shaped modern chemistry between the late 18th and 19th centuries

Introduction: A Clash of Theories and the Birth of Modern Chemistry

What does it mean for a science to have a revolution? For centuries, we've been taught that chemistry had a single, defining revolution at the end of the 18th century, when Antoine Lavoisier overthrew the phlogiston theory and established oxygen as the key to understanding combustion. But what if this familiar narrative is too simplistic? Historical research now suggests that chemistry didn't have just one revolution—it underwent at least three fundamental transformations between the late 18th and 19th centuries.

This article explores these revolutionary periods that transformed chemistry from a mystical art into the quantitative science we know today, reshaping how we understand matter at its most fundamental level.

First Revolution

Lavoisier's Oxygen Theory

Late 18th Century

Second Revolution

Atomic Theory

Early 19th Century

Third Revolution

Structural Chemistry

Mid 19th Century

The Phlogiston Theory and Its Downfall

Before we can understand the revolutions, we must first understand what was revolutionized. For much of the 18th century, the dominant theory in chemistry was phlogiston theory. This theory posited that combustible materials contained a fire-like element called phlogiston, which was released into the air during burning 1 . What we now recognize as combustion was viewed as a decomposition process—when wood burned, it decomposed into phlogiston (which escaped) and ash (which remained) 1 .

Phlogiston Theory
  • Combustion releases phlogiston
  • Burning = Decomposition
  • Substances lose mass when burned
  • Air serves as phlogiston reservoir
  • Qualitative framework
Oxygen Theory
  • Combustion combines with oxygen
  • Burning = Chemical combination
  • Substances gain mass when burned
  • Air provides oxygen for reactions
  • Quantitative, measurement-based

Lavoisier's Revolutionary Experiment

Antoine Lavoisier, often called the "Founder of Modern Chemistry," would not be constrained by the old framework 1 . In a series of meticulous experiments using precise measurements, he demonstrated that combustion involved combination with a component of air, not the release of phlogiston.

Lavoisier's Mercury Experiment
Step 1

Heat mercury in a sealed container

Step 2

Forms red calx (mercury oxide)

Step 3

Mass increases after heating

Step 4

Heat calx strongly to decompose

Step 5

Releases oxygen gas, reforms mercury

Lavoisier's quantitative approach proved that burning was not decomposition but chemical combination—specifically, combination with oxygen from the air 1 . This simple but precise experiment, coupled with his formulation of the law of conservation of mass, marked the first chemical revolution. The balance became chemistry's fundamental instrument, and Lavoisier established a new chemical nomenclature that forms the basis of our modern naming system 1 .

Aspect Phlogiston Theory Lavoisier's Oxygen Theory
Nature of Combustion Decomposition (release of phlogiston) Combination with oxygen
Mass Change During Burning Substances should lose mass Substances gain mass
Role of Air Serves as reservoir for phlogiston Provides oxygen for combination
Conceptual Framework Qualitative Quantitative, based on measurements

The Second Revolution: Atoms and Elements

If Lavoisier's work constituted the first chemical revolution, a second emerged in the early 19th century with the rise of atomic theory and the concept of definite proportions. John Dalton, building on Lavoisier's quantitative approach, proposed that all matter is composed of atoms, and that chemical compounds form when atoms of different elements combine in fixed ratios 6 .

This period was marked by intense debate and experimentation. Joseph Proust's law of definite proportions (1801) stated that chemical compounds always contain the same elements in the same proportion by mass, regardless of how they were prepared 1 . This was contested by Claude Louis Berthollet, who argued for variable composition, but Proust ultimately prevailed after eight years of controversy 1 .

Dalton's atomic theory, published in his "New System of Chemical Philosophy" (1808), provided a theoretical framework that explained why compounds had definite compositions 6 . He proposed that each element consisted of identical atoms, and that chemical compounds formed when atoms of different elements combined in simple whole-number ratios.

The Atomic Theory Toolkit

The acceptance of atomic theory transformed how chemists understood and investigated matter:

Key Concepts
  • Law of Definite Proportions (Proust, 1801): Compounds always have constant composition 1
  • Law of Multiple Proportions (Dalton, 1804): When two elements form different compounds, the mass ratios are small whole numbers 1
  • Avogadro's Hypothesis (1811): Equal volumes of gases at the same temperature and pressure contain equal numbers of molecules
  • Atomic Weights: Berzelius compiled accurate atomic weights for elements, providing essential data for the growing theory 6
Visualizing Atomic Theory
Year Scientist Contribution Impact
1801 Joseph Proust Law of Definite Proportions Established that compounds have fixed composition
1804 John Dalton Law of Multiple Proportions Supported atomic theory through combining ratios
1808 John Dalton Atomic Theory Proposed matter composed of atoms that combine in fixed ratios
1811 Amedeo Avogadro Avogadro's Hypothesis Distinguished between atoms and molecules
1814 Jöns Jakob Berzelius Accurate Atomic Weights Provided essential quantitative data for elements

The Third Revolution: Structure and Organization

The third chemical revolution emerged mid-19th century with the development of structural chemistry and the periodic system. As more elements were discovered and their properties studied, chemists began to recognize patterns that pointed toward an underlying organization of matter.

Friedrich Wöhler's 1828 synthesis of urea from inorganic ammonium cyanate struck a blow against vitalism—the theory that organic compounds could only be produced by living organisms through a "vital force" 2 6 . This discovery helped unify organic and inorganic chemistry and suggested that the same laws governed all matter.

Chemical Structure

August Kekulé and others developed theories of chemical bonding and molecular structure, famously resolving the structure of benzene as a ring 1 4 . This allowed chemists to understand how the arrangement of atoms affected properties.

The Periodic Law

Dmitri Mendeleev and Lothar Meyer independently discovered that when elements are arranged by atomic weight, their properties recur periodically 1 . Mendeleev's genius was in leaving gaps for undiscovered elements and accurately predicting their properties.

The Spectroscope: A Revolutionary Instrument

The 19th century also saw crucial advances in chemical instrumentation. Bunsen and Kirchoff's development of the spectroscope in 1859-60 revolutionized chemical analysis and led to the discovery of seven new elements (rubidium, cesium, thallium, indium, gallium, scandium, and helium) by analyzing their characteristic emission spectra 1 .

Element Prediction Predicted Properties Actual Element (Discovery Year) Actual Properties
"Eka-boron" Atomic weight ~44, oxide formula Eb₂O₃ Scandium (1879) Atomic weight 44.96, oxide formula Sc₂O₃
"Eka-aluminum" Atomic weight ~68, density 5.9 g/cm³ Gallium (1875) Atomic weight 69.7, density 5.9 g/cm³
"Eka-silicon" Atomic weight ~72, density 5.5 g/cm³ Germanium (1886) Atomic weight 72.6, density 5.3 g/cm³
Mendeleev's Predictive Success

The Scientist's Toolkit: Essential Research Materials

The chemical revolutions were enabled by advances in laboratory materials and instruments. Key research reagents and tools included:

Balance

Lavoisier's precise balances enabled quantitative chemistry and the law of conservation of mass 1

Spectroscope

Bunsen and Kirchoff's instrument allowed elemental identification through spectral analysis 1

Voltaic Pile

Alessandro Volta's battery (1800) enabled electrolysis, allowing Davy to isolate elements like sodium and potassium

Mercury

Used in air pumps and for trapping gases in pneumatic experiments 6

Silver Nitrate

Key reagent in early photography and chemical analysis 3

Platinum

Used as a catalyst in contact process for sulfuric acid production 1

Conclusion: Rethinking Chemistry's Revolutions

Viewing chemistry's history through the lens of three revolutions rather than one provides a richer, more accurate narrative of how this fundamental science developed. Each revolution built upon the previous while introducing transformative new concepts:

Lavoisier's Chemical Revolution

Established chemistry as a quantitative science and introduced the conservation of mass.

Dalton's Atomic Revolution

Provided a particulate theory of matter that explained chemical combination.

Structural/Organizational Revolution

Revealed patterns in elemental properties and molecular architecture.

This more nuanced historical view reminds us that scientific progress rarely occurs through a single breakthrough, but through successive waves of conceptual transformation. Each revolution provided new tools, both conceptual and instrumental, that enabled the next advance.

The teaching of chemistry benefits from recognizing these multiple revolutions, as it highlights how scientific knowledge evolves through contested ideas, crucial experiments, and the gradual accumulation of evidence—a process that continues in chemistry laboratories to this day.

References

References